By Priv.-Doz. Dr. Günter Häfelinger (auth.)
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Extra resources for π Complexes of Transition Metals
R'X R ' - C H 2 - C = C H 2 + 2NIX2 I R The synthesis o f o~-santalene from ot,a-dimethylallyl bromide via 7r-allyl nickel complex is an elegant application. 51 J. Tsuji On the other hand, Tsuji, Morikawa, and Takahashi found that zr-allyl palladium complexes react with nucleophiles, such as amines and enamines, and active methylene compounds, such as malonates, with reduction of bivalent palladium to the zero-valent metal 39,4o). This is due to the stability of the reduced species. Pd + CH2(CO2R)2 ' CH2=CH-CH2-CH(CO2R)2 In the dimerization reaction ofbutadiene catalyzed by palladium complexes, nucleophiles (YH), such as amines, alcohols, phenols, carboxylic acids 41-4s), and active methylene compounds 46) are introduced.
The Dithiocarbomates and Related Compounds. Amsterdam: Elsevier Monographs 1962. : Acta Cryst. 19, 619 (1965). : Acta Cryst. 19, 886 (1965). Acta Cryst. 19, 898 (1965). : J. Am. Chem. Soc. 75, 2163 (1953). - lron(II)Diimine and Related Complexes. In: Structure and Bonding, Vol. 9, p. 139. Berlin-Heidelberg-New York: Springer 1971. Figgins, P. , Busch, D. : J. Am. Chem. Soc. 82, 820 (1960). : Angew. Chem. 73, 533 (1961). : Angew. Chem. 76, 76 (1964). Schrauzer, G. : Advan. Organometal. Chem. 2, 17 (1964).
II. a-Bond F o r m a t i o n . . . . . . . . . . 1. Oxidative A d d i t i o n Reactions . . . . . . . 2. Reactivity of a-Bonds . . . . . . . . 3. Oxidative Metal-Metal Bond Cleavage . . . . . 4. Reactions of Transition Metal C o m p o u n d s with Organometallic Compounds . . . . . . . . . . 5. F o r m a t i o n o f Metal Carbonylate Anions from Metal Carbonyls and Their Reactions . . . . . . . . . III. Insertion Reactions . . .
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